looney_tunes Moderator 20 year member
3345 replies
Answer has 3 votes.
Currently voted the best answer.
The first Slavic ruler to take the title of Tsar was Simeon I of Bulgaria, in 893. Even just considering Russia, which is what most people think of, there were a few instances of the title being used even before Ivan III added Tsar of all Russia to the list of titles by which he was to be designated, sometime around 1480.
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